Stratospheric Geoengineering with Sulfate Aerosols
One of the possible impacts of
stratospheric aerosol injections is sulfuric acid deposition. The acidic
deposition would occur as injections of sulfuric acid would combine with water
in the stratosphere forming sulfuric acid which would in turn fall to earth.
The negative effects of sulfur deposition include damage to freshwater fish
populations, reductions in lake bacteria, changes in plant parasite
interactions and changes to forest bird populations.
In 2009, Kravitz et al. investigated the
impacts of sulfuric acid deposition in association with the effects it could
produce on the earth’s surface. The authors assumed all sulfur deposition to be
wet in order to examine the worst possible scenario. The extent to which
sulfate deposition is harmful depends on three things; the amount of sulfur
introduced, the amount of hydrated sulfate and ecosystem sensitivity.
To examine impacts they used a general
circulation model to look at the impacts in different regions and a chemical
model which calculates the sulfur cycle in the stratosphere where the
conversion of SO2 is based upon respective concentrations of SO2 and humidity
values. Over the same time period of 20years, two scenarios were modelled:
- Daily injections of SO2 into the lower stratosphere in the tropics - 5Tg per/year in total
- Daily injections of SO2 into the lower Arctic stratosphere – 3Tg per/year in total
Their results (see figure 1 below) showed that under the 5Tg
scenario, global temperatures could be reduced to levels similar to 1980 and
0.3 degrees of cooling would occur by 2026. Not nearly as impressive, but still
an marked result, changes under the 3Tg scenario would see global average
temperatures immediately reduced to 2000 levels and only 0.3 degrees of warming
would occur by 2026. Sulfur injected over the tropics increased
sulfate deposition across the all of the globe except the tropic due to
poleward transportation. Deposition in the polar regions would also be
particularly apparent. Sulfur injected in the Arctic would lead to deposition
in the Northern Hemisphere.
Figure 1: Annually averaged total sulphate deposition |
The study concluded that sulfur injections
of both 3Tg and 5Tg magnitudes were not significant enough to cause any damage
to the both the regions of the sea and land. This initial study was however flawed
in two ways and consequently in 2010, Kravitz et al. published a follow uppaper to their study correcting these errors.
The first error of the paper was the
calculation for average global surface sulfur emission. When corrected, the
calculation strengthens the conclusion that the additional amount of sulfur
from geo-engineering would be much smaller that current sources. The second
error was their incorrect application of a formula that converts the model
output of sulfate deposition to a form used in critical loading studies.
The incorrect application of the
conversion formula means that figure 2 (see below) their original study needs
to be replaced with the figure below. As you can see the magnitude of the
values change significantly. Despite the changes, the authors still conclude
that acid deposition from geo-engineering would be smaller than the amount
already being experienced in industrialised areas. Furthermore, they hold their
conclusion that everywhere in the world has a significant buffering capacity to
the additional sulfuric acid that would result from geo-engineering except the
most sensitive and pristine areas of the world.
Figure 2: Original model for Tropical SO2 Injections 5 Tg |
Figure 3 - Corrected model for Tropical SO2 Injection 5 Tg |
Even after correcting their errors, the conclusions of Kravitz et al., (2009; 2010) are still the same. Sulfur injections from geo-engineering are not enough to cause any damage except in sensitive, poorly buffered areas; they will not have negative ecosystem impacts. The studies model are accurate however local differences may occur and there may be a need for more significant sulfur injections in the future if GHGs alter atmospheric circulations as aerosol lifetime would be shorter – in which case the model would not serve as accurately. Despite these possibilities, stratospheric aerosol injections are nonetheless a promising geo-engineering technique. The climate cools following sulfur injections and ecosystems are not impacted negatively. As is the case with most geo-engineering techniques their reputation as a taboo topic means more work is often needed to further examine and develop the robustness of techniques. More work on stratospheric aerosols would in my opinion be a good move and a step in the right direction towards fixing climate change!
Thanks for reading!
2009), 'Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols', Journal of Geophysical Research, 114, D14109. (
Kravitz., B (2010), Correction to “Sulfuric acid deposition from stratospheric geo-engineering with sulfate aerosols,” J. Geophys. Res., 115, D16119
2009), 'Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols', Journal of Geophysical Research, 114, D14109. (
Kravitz., B (2010), Correction to “Sulfuric acid deposition from stratospheric geo-engineering with sulfate aerosols,” J. Geophys. Res., 115, D16119
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